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1、Introduction很多文獻(xiàn)已很多文獻(xiàn)已經(jīng)討論過(guò)經(jīng)討論過(guò)了A.Solarenergyconversionbyphotoelectrochemicalcellshasbeenintensivelyinvestigated.(Nature1991353737740)B.Thiswasdemonstratedinanumberofstudiesthatshowedthatcompositeplasmonicmetalsemiconduct

2、photocatalystsachievedsignificantlyhigherratesinvariousphotocatalyticreactionscomparedwiththeirpuresemiconductcounterparts.C.SeveralexcellentreviewsdescribingtheseapplicationsareavailablewedonotdiscussthesetopicsD.Muchwk

3、sofarhasfocusedonwidebgapsemiconductsfwatersplittingfthesakeofchemicalstability.(DOI:10.1038NMAT3151)E.RecentdevelopmentsofLewisacidswatersolubleganometalliccatalystshaveattractedmuchattention.(Chem.Rev.20021023641?3666)

4、F.AninterestingapproachintheuseofzeoliteasawatertolerantsolidacidwasdescribedbyOgawaetal(Chem.Rev.20021023641?3666)G.Considerableresearchefftshavebeendevotedtothedirecttransitionmetalcatalyzedconversionofarylhalidestoary

5、lnitriles.(J.g.Chem.20006579847989)H.TherearemanyexcellentreviewsintheliteraturedealingwiththebasicconceptsofthephotocatalyticprocessthereaderisreferredinparticulartothosebyHoffmanncowkersMillscowkersKamat.(Metaloxidecat

6、alysis19P755)I.NishimiyaTsutsumihavereptedon(proposed)theinfluenceoftheSiAlratioofvariouszeolitesontheacidstrengthwhichwereestimatedbycalimetryusingammonia.(Chem.Rev.20021023641?3666)二、在resultsdiscussion中經(jīng)常會(huì)用到的:如圖所示所示B.A

7、notherinterestingfindingisthatzeoliteswith10memberedringpesshowedhighivities(99%)tocyclohexanolwhereasthosewith12memberedringpessuchasmdeniteproducedlargeamountsofdicyclohexylether.(Chem.Rev.20021023641?3666)C.Itshouldbe

8、pointedoutthatthenanometerscaledistributionofelectrocatalystcentersontheelectrodesurfaceisalsoapredominantfactfhighRelectrocatalyticactivity.D.NotablytheRuIIRhIcomplexespossessingthesameBINAPchiralityfmantipodalaminoacid

9、sasthepredominantproducts.(Angew.Chem.Int.Ed.200241:2008–2022)E.Giventhemultitudeofvarioustransfmationspublisheditisnotewthythatonlyveryfewdistinctactivationmethodshavebeenidentified.(Chem.Soc.Rev.20093821782189)F.Itisim

10、ptanttohighlightthatthesetwodirectingeffectswillleadtodifferentenantiomersoftheproductsevenifboththe“Hbondcatalyst”thecatalystactingbystericshieldinghavethesameabsolutestereochemistry.(Chem.Soc.Rev.20093821782189)G.Itisw

11、thwhilementioningthatthesePPNDscanbeverystablefseveralmonthswithouttheobservationsofanyfloatingprecipitateddotswhichisattributedtotheelectrostaticrepulsionsbetweenthepositivelygePPNDsresultinginelectrostericstabilization

12、.(Adv.Mater.201224:2037–2041)2....仍然是個(gè)挑戰(zhàn)A.ThereistherebyanurgentneedbutitisstillasignificantchallengetorationallydesigndelicatelytailtheelectroactiveMTMOsfadvancedLIBsECsMOBsFCs.(Angew.Chem.Int.Ed.2014531488–1504)B.Howev

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